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wasasurprise,b~cause theheadoftheliquidconvectionpreceded theflame'sIeadingedgebyaproximately1cm[Ito,Masuda,and Saito,191],whichisentirelydiferent仕omAkita'sresult[1972J. To make sure of the ac curacy of the data, we repeated the experimentsseveraltimesandfoundthereproducibilitytobewithin 土 90%. Thus,wepropos巴danewinechanism:theflamespreadin theuIUformspread回 gionisgovemedbytheIiquidconvection[Ito, Masuda,andSaito,191]. However,atthattimewedidnotrealy understandwhyAkita'sshadowgraftresultsweresodiferentfrom ourmresuIts.
Later,HowardRos'sgroupatNASALewisResearchCenter apIiedRainbowSchIierenDeflectometry(RSD)tomeasureliquid convection generated by the spreading flame [MiI Ier and Ros s, 192]. TheyfoundlitleIiquidconvectionaheadoftheflame's leadingedgeintheuniformspreadregion. TheirRSDdatawere similartoAkita'sshadowgraphsanddisagredwithourHIresults. Overthepastthreyears,bothNASAandourgrouphavetriedto understandthereasonsforthedisagrement,butfailedtodosountil a'series of p釘 ametric experiments was completed. In those experiments,theefectsofsixdiferentparameterswereinvestigated: sensitivityofbothRSDandHIsysterns,impurityofpropanol(if any),therelativehumidityoftheair,theambientairtemperaωre, severaldife:ienttypesofignitionmethod,andfinalydiferenttray widths. W efoundthatthe白rstfivepぽ ametershadlit tleinfluenceon thedi5agremen.t However,whenwecheckedthee百ectoftray width(0,5. 1,and2cm)ontheliquidconvection,theleastsusp回 ted parameter,asurprisingresultemerged: the0.5cmwidetrayhada largeIiquidconvectionintheuniformspreadregion,whilethetrays
白atwere1cmand2cmwidehada出inlayerofliquidconvection. Itwas50thinandsmalthatonlyaverysensitivenieasurement techniquecoulddetecti.t Theresultforthe.2・crntrayw部 very similartotheNASA'sresultforthe2・cmtray. A closerlo okattheir RSDresultalsorevealedasmalandthinlayerofIiquidconvection thatwasalwaysaheadoftheflame'sleadingedge. Comparisonof thesefindingsledustotheagrementthatintheuniformspread regionthereisalwaysasmalliquidconvectionindicatingthatthe majQrheattransferisbythatmode. Italsobecamec1eartha.tthe 5hadowgraph [Akita,1972] did not detect the liquid convection becausethesizeoftheIiquidconvect
'fheCurrentProblem NASA'smicrogravitytestresultsshowedthatpulsatingspread
didnotocurineithershaloword田 ppolexperiments[Ros, 194];insteadtheflamewasextinguished,indicatingtheimportance ofthebuoyancye能 ctinthegasphaseonthemechanismof pulsation. SchiIer and Sirignano,using numerical calculations [192],predictedtheexi5tenceofaverysmalcirculationinthegas phaseaheadoftheflame'sleadingedge. Theysugestedthatthe gas~phase circulation,whichisuniqueinthepulsatingspreadand apearswiththeliquid~phase cirω,lation,mayplayanimportantrole
inflamepulsation[192,196]. 百lereareLDVflowmeasurement 142