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Nuclear Reactors and Fuel Cycle | Progress Report  251





               the reactor core and to determine parameters   Neutronic and Thermal-hydraulic
               such as k-effective, neutron flux and power    Analysis of a Device for Irradiation
                                                                                           99
               density. The program SCALE 5.1 was used to     of LEU UAl -Al targets for  Mo
                                                                           x
               find the targets burnup, and the inventory of   Production in the IEA-R1 reactor
               nuclides generated. Neutronic calculations
               showed that the current Brazilian demand       Technetium-99m (  99m Tc), the product of radio-
               of  Mo, 450 Ci per week, and the projected     active decay of molybdenum-99 ( Mo), is one
                  99
                                                                                              99
               future demand of 1000 Ci, can be met by us-    of the most widely used radioisotope in nu-
               ing targets of UAl -Al and U-Ni. The analyzes   clear medicine, covering approximately 80%
                                x
               were realized for the same amount of ura-      of all radiodiagnosis procedures in the world.
               nium present in the targets (20,1 g) and the   Nowadays, Brazil requires an amount of about
               same irradiation conditions. From equation     450 Ci of  Mo per week. Due to the crisis and
                                                                       99
                                                                              99
               {[N * (σ1Φ1 + σ2Φ2 + σ3Φ3 + σ4Φ4) * V * y *    the shortage of  Mo supply chain that has
               (1-e-λt)] / 3.7 * 1010} and from the microscopic   been observed in the world since 2008, IPEN
               fission cross sections produced and collapsed   decided to develop a project to produce  Mo
                                                                                                     99
               into 4 groups by HAMMERTECHNION, it was        through fission of uranium-235. The objective
               possible to calculate the expected results and   of this work was the development of neutronic
               compares them to the results generated with    and thermal-hydraulic calculations to evalu-
               the SCALE 5.1.For UAl -Al and U-Ni plate type   ate the operational safety of a device for  Mo
                                                                                                     99
                                    x
               targets the expected calculations converge to   production to be irradiated in the reactor core
               values very close to those performed by the    IEA-R1 at 5 MW. In this device, ten targets of
               SCALE, but for the U-Ni cylindrical target, the   UAl -Al dispersion fuel with low enriched
                                                                  x
               results were inconsistent. The inconsistency   uranium (LEU) and density of 2.889 gU/cm³
               was due to the fact that the HAMMERTECH-       were placed. For the neutronic calculations,
               NION does not have a module for calculating    the computer codes HAMMER-TECHNION
               self-shielding, which makes it unsuitable      and CITATION were utilized and the maxi-
               for this analysis. To solve the problem, the   mum temperatures reached in the targets
               software package AMPX from the Oak Ridge       were calculated with the code MTRCR-IEAR1.
               National Laboratory was used to generate       The analysis demonstrated that the device
               the cross sections of the homogenized cell     irradiation will occur without adverse conse-
               (aluminum radiator + U-Ni cylindrical target   quences to the operation of the reactor. The
               + cooling channels) of the U-Ni cylindrical    total amount of  Mo was calculated with
                                                                               99
               target. This program package contains the      the program SCALE, obtaining an activity of
               module Rolaids(,) which executes an integral   620 Ci for 3 days irradiation, 831.96 Ci for 5
               transport calculation to handle the effect of   days and, after 7 days irradiation, the activity
               self-shielding in multi- regions. The programs   was 958.3 Ci.
               SCALE 5.1 and MCNP 5 were utilized for cal-
               culation the cross sections of the reactor core   Study of necessary equipment for
               materials, the 3D modeling of the core and     cogeneration viability in commercial
               to determine parameters such as k-effective,   installations at concession area of
               the neutron flux and power density. The cal-   the São Paulo Gas Company
               culations were compared with each other to
               ensure consistency of methodology.             This study aims to identify the characteris-
                                                              tics of the equipment, to generate the energy
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